Insight into Acid-Base Nucleation Experiments by Comparison of the Chemical Composition of Positive, Negative, and Neutral Clusters
Identifieur interne : 000325 ( France/Analysis ); précédent : 000324; suivant : 000326Insight into Acid-Base Nucleation Experiments by Comparison of the Chemical Composition of Positive, Negative, and Neutral Clusters
Auteurs : Federico Bianchi [Suisse] ; Arnaud P. Praplan [Finlande] ; Nina Sarnela [Finlande] ; Josef Dommen [Suisse] ; Andreas Kürten [Allemagne] ; Ismael K. Ortega [France] ; Siegfried Schobesberger [Finlande] ; Heikki Junninen [Finlande] ; Mario Simon [Allemagne] ; Jasmin Tröstl [Suisse] ; Tuija Jokinen [Finlande] ; Mikko Sipil [Finlande] ; Alexey Adamov [Finlande] ; Antonio Amonm [Portugal] ; Joao Almeida [Suisse] ; Martin Breitenlechner [Autriche] ; Jonathan Duplissy [Finlande, Suisse] ; Sebastian Ehrhart [Suisse] ; Richard C. Flagan [États-Unis] ; Alessandro Franchin [Finlande] ; Jani Hakala [Finlande] ; Armin Hansel [Autriche] ; Martin Heinritzi [Allemagne, Autriche] ; Juha Kangasluoma [Finlande] ; Helmi Keskinen [Finlande] ; JAESEOK KIM [Finlande] ; Jasper Kirkby [Allemagne, Suisse] ; Ari Laaksonen [Suisse, Finlande] ; Michael J. Lawler [Finlande, États-Unis] ; Katrianne Lehtipalo [Finlande] ; Markus Leiminger [Allemagne] ; Vladimir Makhmutov [Russie] ; Serge Mathot [Suisse] ; Antti Onnela [Suisse] ; Tuukka Pet J [Finlande] ; Francesco Riccobono [Suisse] ; Matti P. Rissanen [Finlande] ; Linda Rondo [Allemagne] ; Ant Nio Tome [Portugal] ; Annele Virtanen [Suisse] ; Yrjö Viisanen [Finlande] ; Christina Williamson [Allemagne] ; Daniela Wimmer [Finlande, Allemagne] ; Paul M. Winkler [Autriche] ; PENGLIN YE [États-Unis] ; Joachim Curtius [Allemagne] ; Markku Kuimala [Finlande] ; Douglas R. Worsnop [Finlande, États-Unis] ; Neil M. Donahue [États-Unis] ; Urs Baltensperger [Suisse]Source :
- Environmental science & technology [ 0013-936X ] ; 2014.
Descripteurs français
- Pascal (Inist)
- Wicri :
- topic : Aérosol.
English descriptors
- KwdEn :
Abstract
We investigated the nucleation of sulfuric acid together with two bases (ammonia and dimethylamine), at the CLOUD chamber at CERN. The chemical composition of positive, negative, and neutral clusters was studied using three Atmospheric Pressure interface-Time Of Flight (APi-TOF) mass spectrometers: two were operated in positive and negative mode to detect the chamber ions, while the third was equipped with a nitrate ion chemical ionization source allowing detection of neutral clusters. Taking into account the possible fragmentation that can happen during the charging of the ions or within the first stage of the mass spectrometer, the cluster formation proceeded via essentially one-to-one acid-base addition for all of the clusters, independent of the type of the base. For the positive clusters, the charge is carried by one excess protonated base, while for the negative clusters it is carried by a deprotonated add; the same is true for the neutral clusters after these have been ionized During the experiments involving sulfuric acid and dimethylamine, it was possible to study the appearance time for all the clusters (positive, negative, and neutral). It appeared that, after the formation of the clusters containing three molecules of sulfuric acid, the clusters grow at a similar speed, independent of their charge. The growth rate is then probably limited by the arrival rate of sulfuric acid or cluster-cluster collision.
Affiliations:
- Allemagne, Autriche, Finlande, France, Portugal, Russie, Suisse, États-Unis
- District de Darmstadt, District fédéral central, Hesse (Land), Pennsylvanie, Uusimaa, Vienne (Autriche)
- Francfort-sur-le-Main, Helsinki, Moscou, Pittsburgh, Vienne (Autriche)
- Université Carnegie-Mellon, Université d'Helsinki
Links toward previous steps (curation, corpus...)
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Pascal:15-0038329Le document en format XML
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Lisboa and U. Beira Interior</s1><s2>Lisbon 1749</s2><s3>PRT</s3><sZ>14 aut.</sZ><sZ>39 aut.</sZ></inist:fA14><country>Portugal</country><wicri:noRegion>Lisbon 1749</wicri:noRegion></affiliation></author><author><name sortKey="Almeida, Joao" sort="Almeida, Joao" uniqKey="Almeida J" first="Joao" last="Almeida">Joao Almeida</name><affiliation wicri:level="1"><inist:fA14 i1="06"><s1>CERN</s1><s2>Geneva 1211</s2><s3>CHE</s3><sZ>15 aut.</sZ><sZ>17 aut.</sZ><sZ>18 aut.</sZ><sZ>27 aut.</sZ><sZ>33 aut.</sZ><sZ>34 aut.</sZ></inist:fA14><country>Suisse</country><wicri:noRegion>CERN</wicri:noRegion></affiliation></author><author><name sortKey="Breitenlechner, Martin" sort="Breitenlechner, Martin" uniqKey="Breitenlechner M" first="Martin" last="Breitenlechner">Martin Breitenlechner</name><affiliation wicri:level="1"><inist:fA14 i1="07"><s1>University of Innsbruck</s1><s2>Innsbruck 6020</s2><s3>AUT</s3><sZ>16 aut.</sZ><sZ>22 aut.</sZ><sZ>23 aut.</sZ></inist:fA14><country>Autriche</country><wicri:noRegion>University of Innsbruck</wicri:noRegion></affiliation><affiliation wicri:level="1"><inist:fA14 i1="08"><s1>IONICON Analytik GmbH</s1><s2>Innsbruck 6020</s2><s3>AUT</s3><sZ>16 aut.</sZ><sZ>22 aut.</sZ></inist:fA14><country>Autriche</country><wicri:noRegion>IONICON Analytik GmbH</wicri:noRegion></affiliation></author><author><name sortKey="Duplissy, Jonathan" sort="Duplissy, Jonathan" uniqKey="Duplissy J" first="Jonathan" last="Duplissy">Jonathan Duplissy</name><affiliation wicri:level="4"><inist:fA14 i1="02"><s1>Departrnent of Physics, University of Helsinki</s1><s2>Helsinki 00014</s2><s3>FIN</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>7 aut.</sZ><sZ>8 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>17 aut.</sZ><sZ>20 aut.</sZ><sZ>21 aut.</sZ><sZ>24 aut.</sZ><sZ>30 aut.</sZ><sZ>35 aut.</sZ><sZ>37 aut.</sZ><sZ>43 aut.</sZ><sZ>47 aut.</sZ><sZ>48 aut.</sZ></inist:fA14><country>Finlande</country><placeName><settlement type="city">Helsinki</settlement><region type="région" nuts="2">Uusimaa</region></placeName><orgName type="university">Université d'Helsinki</orgName></affiliation><affiliation wicri:level="1"><inist:fA14 i1="06"><s1>CERN</s1><s2>Geneva 1211</s2><s3>CHE</s3><sZ>15 aut.</sZ><sZ>17 aut.</sZ><sZ>18 aut.</sZ><sZ>27 aut.</sZ><sZ>33 aut.</sZ><sZ>34 aut.</sZ></inist:fA14><country>Suisse</country><wicri:noRegion>CERN</wicri:noRegion></affiliation><affiliation wicri:level="1"><inist:fA14 i1="09"><s1>Helsinki Institute of Physics</s1><s2>Helsinki 00014</s2><s3>FIN</s3><sZ>17 aut.</sZ></inist:fA14><country>Finlande</country><wicri:noRegion>Helsinki Institute of Physics</wicri:noRegion></affiliation></author><author><name sortKey="Ehrhart, Sebastian" sort="Ehrhart, Sebastian" uniqKey="Ehrhart S" first="Sebastian" last="Ehrhart">Sebastian Ehrhart</name><affiliation wicri:level="1"><inist:fA14 i1="06"><s1>CERN</s1><s2>Geneva 1211</s2><s3>CHE</s3><sZ>15 aut.</sZ><sZ>17 aut.</sZ><sZ>18 aut.</sZ><sZ>27 aut.</sZ><sZ>33 aut.</sZ><sZ>34 aut.</sZ></inist:fA14><country>Suisse</country><wicri:noRegion>CERN</wicri:noRegion></affiliation></author><author><name sortKey="Flagan, Richard C" sort="Flagan, Richard C" uniqKey="Flagan R" first="Richard C." last="Flagan">Richard C. Flagan</name><affiliation wicri:level="1"><inist:fA14 i1="10"><s1>Califomia Institute of Technology</s1><s2>Pasadena, California 91125</s2><s3>USA</s3><sZ>19 aut.</sZ></inist:fA14><country>États-Unis</country><wicri:noRegion>Califomia Institute of Technology</wicri:noRegion></affiliation></author><author><name sortKey="Franchin, Alessandro" sort="Franchin, Alessandro" uniqKey="Franchin A" first="Alessandro" last="Franchin">Alessandro Franchin</name><affiliation wicri:level="4"><inist:fA14 i1="02"><s1>Departrnent of Physics, University of Helsinki</s1><s2>Helsinki 00014</s2><s3>FIN</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>7 aut.</sZ><sZ>8 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>17 aut.</sZ><sZ>20 aut.</sZ><sZ>21 aut.</sZ><sZ>24 aut.</sZ><sZ>30 aut.</sZ><sZ>35 aut.</sZ><sZ>37 aut.</sZ><sZ>43 aut.</sZ><sZ>47 aut.</sZ><sZ>48 aut.</sZ></inist:fA14><country>Finlande</country><placeName><settlement type="city">Helsinki</settlement><region type="région" 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Hansel</name><affiliation wicri:level="1"><inist:fA14 i1="07"><s1>University of Innsbruck</s1><s2>Innsbruck 6020</s2><s3>AUT</s3><sZ>16 aut.</sZ><sZ>22 aut.</sZ><sZ>23 aut.</sZ></inist:fA14><country>Autriche</country><wicri:noRegion>University of Innsbruck</wicri:noRegion></affiliation><affiliation wicri:level="1"><inist:fA14 i1="08"><s1>IONICON Analytik GmbH</s1><s2>Innsbruck 6020</s2><s3>AUT</s3><sZ>16 aut.</sZ><sZ>22 aut.</sZ></inist:fA14><country>Autriche</country><wicri:noRegion>IONICON Analytik GmbH</wicri:noRegion></affiliation></author><author><name sortKey="Heinritzi, Martin" sort="Heinritzi, Martin" uniqKey="Heinritzi M" first="Martin" last="Heinritzi">Martin Heinritzi</name><affiliation wicri:level="3"><inist:fA14 i1="03"><s1>Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt am Main</s1><s2>Frankfurt am Main 60438</s2><s3>DEU</s3><sZ>5 aut.</sZ><sZ>9 aut.</sZ><sZ>23 aut.</sZ><sZ>27 aut.</sZ><sZ>31 aut.</sZ><sZ>38 aut.</sZ><sZ>42 aut.</sZ><sZ>43 aut.</sZ><sZ>46 aut.</sZ></inist:fA14><country>Allemagne</country><placeName><region type="land" nuts="1">Hesse (Land)</region><region type="district" nuts="2">District de Darmstadt</region><settlement type="city">Francfort-sur-le-Main</settlement></placeName></affiliation><affiliation wicri:level="1"><inist:fA14 i1="07"><s1>University of Innsbruck</s1><s2>Innsbruck 6020</s2><s3>AUT</s3><sZ>16 aut.</sZ><sZ>22 aut.</sZ><sZ>23 aut.</sZ></inist:fA14><country>Autriche</country><wicri:noRegion>University of Innsbruck</wicri:noRegion></affiliation></author><author><name sortKey="Kangasluoma, Juha" sort="Kangasluoma, Juha" uniqKey="Kangasluoma J" first="Juha" last="Kangasluoma">Juha Kangasluoma</name><affiliation wicri:level="4"><inist:fA14 i1="02"><s1>Departrnent of Physics, University of Helsinki</s1><s2>Helsinki 00014</s2><s3>FIN</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>7 aut.</sZ><sZ>8 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>17 aut.</sZ><sZ>20 aut.</sZ><sZ>21 aut.</sZ><sZ>24 aut.</sZ><sZ>30 aut.</sZ><sZ>35 aut.</sZ><sZ>37 aut.</sZ><sZ>43 aut.</sZ><sZ>47 aut.</sZ><sZ>48 aut.</sZ></inist:fA14><country>Finlande</country><placeName><settlement type="city">Helsinki</settlement><region type="région" nuts="2">Uusimaa</region></placeName><orgName type="university">Université d'Helsinki</orgName></affiliation></author><author><name sortKey="Keskinen, Helmi" sort="Keskinen, Helmi" uniqKey="Keskinen H" first="Helmi" last="Keskinen">Helmi Keskinen</name><affiliation wicri:level="1"><inist:fA14 i1="11"><s1>Department of Applied Physics, University of Eastern Finland</s1><s2>Kuopio 70211</s2><s3>FIN</s3><sZ>25 aut.</sZ><sZ>26 aut.</sZ><sZ>29 aut.</sZ></inist:fA14><country>Finlande</country><wicri:noRegion>Kuopio 70211</wicri:noRegion></affiliation></author><author><name sortKey="Jaeseok Kim" sort="Jaeseok Kim" uniqKey="Jaeseok Kim" last="Jaeseok Kim">JAESEOK KIM</name><affiliation wicri:level="1"><inist:fA14 i1="11"><s1>Department of Applied Physics, University of Eastern Finland</s1><s2>Kuopio 70211</s2><s3>FIN</s3><sZ>25 aut.</sZ><sZ>26 aut.</sZ><sZ>29 aut.</sZ></inist:fA14><country>Finlande</country><wicri:noRegion>Kuopio 70211</wicri:noRegion></affiliation></author><author><name sortKey="Kirkby, Jasper" sort="Kirkby, Jasper" uniqKey="Kirkby J" first="Jasper" last="Kirkby">Jasper Kirkby</name><affiliation wicri:level="3"><inist:fA14 i1="03"><s1>Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt am Main</s1><s2>Frankfurt am Main 60438</s2><s3>DEU</s3><sZ>5 aut.</sZ><sZ>9 aut.</sZ><sZ>23 aut.</sZ><sZ>27 aut.</sZ><sZ>31 aut.</sZ><sZ>38 aut.</sZ><sZ>42 aut.</sZ><sZ>43 aut.</sZ><sZ>46 aut.</sZ></inist:fA14><country>Allemagne</country><placeName><region type="land" nuts="1">Hesse (Land)</region><region type="district" nuts="2">District de Darmstadt</region><settlement type="city">Francfort-sur-le-Main</settlement></placeName></affiliation><affiliation wicri:level="1"><inist:fA14 i1="06"><s1>CERN</s1><s2>Geneva 1211</s2><s3>CHE</s3><sZ>15 aut.</sZ><sZ>17 aut.</sZ><sZ>18 aut.</sZ><sZ>27 aut.</sZ><sZ>33 aut.</sZ><sZ>34 aut.</sZ></inist:fA14><country>Suisse</country><wicri:noRegion>CERN</wicri:noRegion></affiliation></author><author><name sortKey="Laaksonen, Ari" sort="Laaksonen, Ari" uniqKey="Laaksonen A" first="Ari" last="Laaksonen">Ari Laaksonen</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Laboratory of Atmospheric Chemistry, Paul Scherrer Institute</s1><s2>Villigen 5232</s2><s3>CHE</s3><sZ>1 aut.</sZ><sZ>4 aut.</sZ><sZ>10 aut.</sZ><sZ>28 aut.</sZ><sZ>36 aut.</sZ><sZ>40 aut.</sZ><sZ>50 aut.</sZ></inist:fA14><country>Suisse</country><wicri:noRegion>Villigen 5232</wicri:noRegion></affiliation><affiliation wicri:level="1"><inist:fA14 i1="15"><s1>Finnish Meteorological Institute</s1><s2>Helsinki 00101</s2><s3>FIN</s3><sZ>28 aut.</sZ><sZ>41 aut.</sZ></inist:fA14><country>Finlande</country><wicri:noRegion>Finnish Meteorological Institute</wicri:noRegion></affiliation></author><author><name sortKey="Lawler, Michael J" sort="Lawler, Michael J" uniqKey="Lawler M" first="Michael J." last="Lawler">Michael J. Lawler</name><affiliation wicri:level="1"><inist:fA14 i1="11"><s1>Department of Applied Physics, University of Eastern Finland</s1><s2>Kuopio 70211</s2><s3>FIN</s3><sZ>25 aut.</sZ><sZ>26 aut.</sZ><sZ>29 aut.</sZ></inist:fA14><country>Finlande</country><wicri:noRegion>Kuopio 70211</wicri:noRegion></affiliation><affiliation wicri:level="1"><inist:fA14 i1="12"><s1>Atmospheric Chemistry Division, National Center for Atmospheric Research</s1><s2>Boulder, Colorado 80301</s2><s3>USA</s3><sZ>29 aut.</sZ></inist:fA14><country>États-Unis</country><wicri:noRegion>Boulder, Colorado 80301</wicri:noRegion></affiliation></author><author><name sortKey="Lehtipalo, Katrianne" sort="Lehtipalo, Katrianne" uniqKey="Lehtipalo K" first="Katrianne" last="Lehtipalo">Katrianne Lehtipalo</name><affiliation wicri:level="4"><inist:fA14 i1="02"><s1>Departrnent of Physics, University of Helsinki</s1><s2>Helsinki 00014</s2><s3>FIN</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>7 aut.</sZ><sZ>8 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>17 aut.</sZ><sZ>20 aut.</sZ><sZ>21 aut.</sZ><sZ>24 aut.</sZ><sZ>30 aut.</sZ><sZ>35 aut.</sZ><sZ>37 aut.</sZ><sZ>43 aut.</sZ><sZ>47 aut.</sZ><sZ>48 aut.</sZ></inist:fA14><country>Finlande</country><placeName><settlement type="city">Helsinki</settlement><region type="région" nuts="2">Uusimaa</region></placeName><orgName type="university">Université d'Helsinki</orgName></affiliation><affiliation wicri:level="1"><inist:fA14 i1="13"><s1>Airmodus Ltd</s1><s2>Helsinki 00560</s2><s3>FIN</s3><sZ>30 aut.</sZ></inist:fA14><country>Finlande</country><wicri:noRegion>Airmodus Ltd</wicri:noRegion></affiliation></author><author><name sortKey="Leiminger, Markus" sort="Leiminger, Markus" uniqKey="Leiminger M" first="Markus" last="Leiminger">Markus Leiminger</name><affiliation wicri:level="3"><inist:fA14 i1="03"><s1>Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt am Main</s1><s2>Frankfurt am Main 60438</s2><s3>DEU</s3><sZ>5 aut.</sZ><sZ>9 aut.</sZ><sZ>23 aut.</sZ><sZ>27 aut.</sZ><sZ>31 aut.</sZ><sZ>38 aut.</sZ><sZ>42 aut.</sZ><sZ>43 aut.</sZ><sZ>46 aut.</sZ></inist:fA14><country>Allemagne</country><placeName><region type="land" nuts="1">Hesse (Land)</region><region type="district" nuts="2">District de Darmstadt</region><settlement type="city">Francfort-sur-le-Main</settlement></placeName></affiliation></author><author><name sortKey="Makhmutov, Vladimir" sort="Makhmutov, Vladimir" uniqKey="Makhmutov V" first="Vladimir" last="Makhmutov">Vladimir Makhmutov</name><affiliation wicri:level="1"><inist:fA14 i1="14"><s1>Lebedev Physical Institute RAS, Leninsky prospekt</s1><s2>Moscow 119991</s2><s3>RUS</s3><sZ>32 aut.</sZ></inist:fA14><country>Russie</country><placeName><settlement type="city">Moscou</settlement><region>District fédéral central</region></placeName></affiliation></author><author><name sortKey="Mathot, Serge" sort="Mathot, Serge" uniqKey="Mathot S" first="Serge" last="Mathot">Serge Mathot</name><affiliation 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aut.</sZ><sZ>8 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>17 aut.</sZ><sZ>20 aut.</sZ><sZ>21 aut.</sZ><sZ>24 aut.</sZ><sZ>30 aut.</sZ><sZ>35 aut.</sZ><sZ>37 aut.</sZ><sZ>43 aut.</sZ><sZ>47 aut.</sZ><sZ>48 aut.</sZ></inist:fA14><country>Finlande</country><placeName><settlement type="city">Helsinki</settlement><region type="région" nuts="2">Uusimaa</region></placeName><orgName type="university">Université d'Helsinki</orgName></affiliation></author><author><name sortKey="Riccobono, Francesco" sort="Riccobono, Francesco" uniqKey="Riccobono F" first="Francesco" last="Riccobono">Francesco Riccobono</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Laboratory of Atmospheric Chemistry, Paul Scherrer Institute</s1><s2>Villigen 5232</s2><s3>CHE</s3><sZ>1 aut.</sZ><sZ>4 aut.</sZ><sZ>10 aut.</sZ><sZ>28 aut.</sZ><sZ>36 aut.</sZ><sZ>40 aut.</sZ><sZ>50 aut.</sZ></inist:fA14><country>Suisse</country><wicri:noRegion>Villigen 5232</wicri:noRegion></affiliation></author><author><name sortKey="Rissanen, Matti P" sort="Rissanen, Matti P" uniqKey="Rissanen M" first="Matti P." last="Rissanen">Matti P. Rissanen</name><affiliation wicri:level="4"><inist:fA14 i1="02"><s1>Departrnent of Physics, University of Helsinki</s1><s2>Helsinki 00014</s2><s3>FIN</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>7 aut.</sZ><sZ>8 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>17 aut.</sZ><sZ>20 aut.</sZ><sZ>21 aut.</sZ><sZ>24 aut.</sZ><sZ>30 aut.</sZ><sZ>35 aut.</sZ><sZ>37 aut.</sZ><sZ>43 aut.</sZ><sZ>47 aut.</sZ><sZ>48 aut.</sZ></inist:fA14><country>Finlande</country><placeName><settlement type="city">Helsinki</settlement><region type="région" nuts="2">Uusimaa</region></placeName><orgName type="university">Université d'Helsinki</orgName></affiliation></author><author><name sortKey="Rondo, Linda" sort="Rondo, Linda" uniqKey="Rondo L" first="Linda" last="Rondo">Linda Rondo</name><affiliation wicri:level="3"><inist:fA14 i1="03"><s1>Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt am Main</s1><s2>Frankfurt am Main 60438</s2><s3>DEU</s3><sZ>5 aut.</sZ><sZ>9 aut.</sZ><sZ>23 aut.</sZ><sZ>27 aut.</sZ><sZ>31 aut.</sZ><sZ>38 aut.</sZ><sZ>42 aut.</sZ><sZ>43 aut.</sZ><sZ>46 aut.</sZ></inist:fA14><country>Allemagne</country><placeName><region type="land" nuts="1">Hesse (Land)</region><region type="district" nuts="2">District de Darmstadt</region><settlement type="city">Francfort-sur-le-Main</settlement></placeName></affiliation></author><author><name sortKey="Tome, Ant Nio" sort="Tome, Ant Nio" uniqKey="Tome A" first="Ant Nio" last="Tome">Ant Nio Tome</name><affiliation wicri:level="1"><inist:fA14 i1="05"><s1>CENTRA-SIM, U. Lisboa and U. Beira Interior</s1><s2>Lisbon 1749</s2><s3>PRT</s3><sZ>14 aut.</sZ><sZ>39 aut.</sZ></inist:fA14><country>Portugal</country><wicri:noRegion>Lisbon 1749</wicri:noRegion></affiliation></author><author><name sortKey="Virtanen, Annele" sort="Virtanen, Annele" uniqKey="Virtanen A" first="Annele" last="Virtanen">Annele Virtanen</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Laboratory of Atmospheric Chemistry, Paul Scherrer Institute</s1><s2>Villigen 5232</s2><s3>CHE</s3><sZ>1 aut.</sZ><sZ>4 aut.</sZ><sZ>10 aut.</sZ><sZ>28 aut.</sZ><sZ>36 aut.</sZ><sZ>40 aut.</sZ><sZ>50 aut.</sZ></inist:fA14><country>Suisse</country><wicri:noRegion>Villigen 5232</wicri:noRegion></affiliation></author><author><name sortKey="Viisanen, Yrjo" sort="Viisanen, Yrjo" uniqKey="Viisanen Y" first="Yrjö" last="Viisanen">Yrjö Viisanen</name><affiliation wicri:level="1"><inist:fA14 i1="15"><s1>Finnish Meteorological Institute</s1><s2>Helsinki 00101</s2><s3>FIN</s3><sZ>28 aut.</sZ><sZ>41 aut.</sZ></inist:fA14><country>Finlande</country><wicri:noRegion>Finnish Meteorological Institute</wicri:noRegion></affiliation></author><author><name sortKey="Williamson, Christina" sort="Williamson, Christina" uniqKey="Williamson C" first="Christina" last="Williamson">Christina Williamson</name><affiliation wicri:level="3"><inist:fA14 i1="03"><s1>Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt am Main</s1><s2>Frankfurt am Main 60438</s2><s3>DEU</s3><sZ>5 aut.</sZ><sZ>9 aut.</sZ><sZ>23 aut.</sZ><sZ>27 aut.</sZ><sZ>31 aut.</sZ><sZ>38 aut.</sZ><sZ>42 aut.</sZ><sZ>43 aut.</sZ><sZ>46 aut.</sZ></inist:fA14><country>Allemagne</country><placeName><region type="land" nuts="1">Hesse (Land)</region><region type="district" nuts="2">District de Darmstadt</region><settlement type="city">Francfort-sur-le-Main</settlement></placeName></affiliation></author><author><name sortKey="Wimmer, Daniela" sort="Wimmer, Daniela" uniqKey="Wimmer D" first="Daniela" last="Wimmer">Daniela Wimmer</name><affiliation wicri:level="4"><inist:fA14 i1="02"><s1>Departrnent of Physics, University of Helsinki</s1><s2>Helsinki 00014</s2><s3>FIN</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>7 aut.</sZ><sZ>8 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>17 aut.</sZ><sZ>20 aut.</sZ><sZ>21 aut.</sZ><sZ>24 aut.</sZ><sZ>30 aut.</sZ><sZ>35 aut.</sZ><sZ>37 aut.</sZ><sZ>43 aut.</sZ><sZ>47 aut.</sZ><sZ>48 aut.</sZ></inist:fA14><country>Finlande</country><placeName><settlement type="city">Helsinki</settlement><region type="région" nuts="2">Uusimaa</region></placeName><orgName type="university">Université d'Helsinki</orgName></affiliation><affiliation wicri:level="3"><inist:fA14 i1="03"><s1>Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt am Main</s1><s2>Frankfurt am Main 60438</s2><s3>DEU</s3><sZ>5 aut.</sZ><sZ>9 aut.</sZ><sZ>23 aut.</sZ><sZ>27 aut.</sZ><sZ>31 aut.</sZ><sZ>38 aut.</sZ><sZ>42 aut.</sZ><sZ>43 aut.</sZ><sZ>46 aut.</sZ></inist:fA14><country>Allemagne</country><placeName><region type="land" nuts="1">Hesse (Land)</region><region type="district" nuts="2">District de Darmstadt</region><settlement type="city">Francfort-sur-le-Main</settlement></placeName></affiliation></author><author><name sortKey="Winkler, Paul M" sort="Winkler, Paul M" uniqKey="Winkler P" first="Paul M." last="Winkler">Paul M. Winkler</name><affiliation wicri:level="1"><inist:fA14 i1="16"><s1>Faculty of Physics, University of Vienna</s1><s2>Vienna 1090</s2><s3>AUT</s3><sZ>44 aut.</sZ></inist:fA14><country>Autriche</country><placeName><settlement type="city">Vienne (Autriche)</settlement><region nuts="2" type="province">Vienne (Autriche)</region></placeName></affiliation></author><author><name sortKey="Penglin Ye" sort="Penglin Ye" uniqKey="Penglin Ye" last="Penglin Ye">PENGLIN YE</name><affiliation wicri:level="4"><inist:fA14 i1="17"><s1>Center for Atmospheric Particle Studies, Carnegie Mellon University</s1><s2>Pittsburgh, Pennsylvania 15213</s2><s3>USA</s3><sZ>45 aut.</sZ><sZ>49 aut.</sZ></inist:fA14><country>États-Unis</country><placeName><settlement type="city">Pittsburgh</settlement><region type="state">Pennsylvanie</region></placeName><orgName type="university">Université Carnegie-Mellon</orgName></affiliation></author><author><name sortKey="Curtius, Joachim" sort="Curtius, Joachim" uniqKey="Curtius J" first="Joachim" last="Curtius">Joachim Curtius</name><affiliation wicri:level="3"><inist:fA14 i1="03"><s1>Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt am Main</s1><s2>Frankfurt am Main 60438</s2><s3>DEU</s3><sZ>5 aut.</sZ><sZ>9 aut.</sZ><sZ>23 aut.</sZ><sZ>27 aut.</sZ><sZ>31 aut.</sZ><sZ>38 aut.</sZ><sZ>42 aut.</sZ><sZ>43 aut.</sZ><sZ>46 aut.</sZ></inist:fA14><country>Allemagne</country><placeName><region type="land" nuts="1">Hesse (Land)</region><region type="district" nuts="2">District de Darmstadt</region><settlement type="city">Francfort-sur-le-Main</settlement></placeName></affiliation></author><author><name sortKey="Kuimala, Markku" sort="Kuimala, Markku" uniqKey="Kuimala M" first="Markku" last="Kuimala">Markku Kuimala</name><affiliation wicri:level="4"><inist:fA14 i1="02"><s1>Departrnent of Physics, University of Helsinki</s1><s2>Helsinki 00014</s2><s3>FIN</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>7 aut.</sZ><sZ>8 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>17 aut.</sZ><sZ>20 aut.</sZ><sZ>21 aut.</sZ><sZ>24 aut.</sZ><sZ>30 aut.</sZ><sZ>35 aut.</sZ><sZ>37 aut.</sZ><sZ>43 aut.</sZ><sZ>47 aut.</sZ><sZ>48 aut.</sZ></inist:fA14><country>Finlande</country><placeName><settlement type="city">Helsinki</settlement><region type="région" nuts="2">Uusimaa</region></placeName><orgName type="university">Université d'Helsinki</orgName></affiliation></author><author><name sortKey="Worsnop, Douglas R" sort="Worsnop, Douglas R" uniqKey="Worsnop D" first="Douglas R." last="Worsnop">Douglas R. Worsnop</name><affiliation wicri:level="4"><inist:fA14 i1="02"><s1>Departrnent of Physics, University of Helsinki</s1><s2>Helsinki 00014</s2><s3>FIN</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>7 aut.</sZ><sZ>8 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>17 aut.</sZ><sZ>20 aut.</sZ><sZ>21 aut.</sZ><sZ>24 aut.</sZ><sZ>30 aut.</sZ><sZ>35 aut.</sZ><sZ>37 aut.</sZ><sZ>43 aut.</sZ><sZ>47 aut.</sZ><sZ>48 aut.</sZ></inist:fA14><country>Finlande</country><placeName><settlement type="city">Helsinki</settlement><region type="région" nuts="2">Uusimaa</region></placeName><orgName type="university">Université d'Helsinki</orgName></affiliation><affiliation wicri:level="1"><inist:fA14 i1="18"><s1>Aerodyne Research Inc.</s1><s2>Billerica, Massachusetts 01821</s2><s3>USA</s3><sZ>48 aut.</sZ></inist:fA14><country>États-Unis</country><wicri:noRegion>Aerodyne Research Inc.</wicri:noRegion></affiliation></author><author><name sortKey="Donahue, Neil M" sort="Donahue, Neil M" uniqKey="Donahue N" first="Neil M." last="Donahue">Neil M. Donahue</name><affiliation wicri:level="4"><inist:fA14 i1="17"><s1>Center for Atmospheric Particle Studies, Carnegie Mellon University</s1><s2>Pittsburgh, Pennsylvania 15213</s2><s3>USA</s3><sZ>45 aut.</sZ><sZ>49 aut.</sZ></inist:fA14><country>États-Unis</country><placeName><settlement type="city">Pittsburgh</settlement><region type="state">Pennsylvanie</region></placeName><orgName type="university">Université Carnegie-Mellon</orgName></affiliation></author><author><name sortKey="Baltensperger, Urs" sort="Baltensperger, Urs" uniqKey="Baltensperger U" first="Urs" last="Baltensperger">Urs Baltensperger</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Laboratory of Atmospheric Chemistry, Paul Scherrer Institute</s1><s2>Villigen 5232</s2><s3>CHE</s3><sZ>1 aut.</sZ><sZ>4 aut.</sZ><sZ>10 aut.</sZ><sZ>28 aut.</sZ><sZ>36 aut.</sZ><sZ>40 aut.</sZ><sZ>50 aut.</sZ></inist:fA14><country>Suisse</country><wicri:noRegion>Villigen 5232</wicri:noRegion></affiliation></author></titleStmt><publicationStmt><idno type="wicri:source">INIST</idno><idno type="inist">15-0038329</idno><date when="2014">2014</date><idno type="stanalyst">PASCAL 15-0038329 INIST</idno><idno type="RBID">Pascal:15-0038329</idno><idno type="wicri:Area/PascalFrancis/Corpus">000056</idno><idno type="wicri:Area/PascalFrancis/Curation">004538</idno><idno type="wicri:Area/PascalFrancis/Checkpoint">000711</idno><idno type="wicri:explorRef" wicri:stream="PascalFrancis" wicri:step="Checkpoint">000711</idno><idno type="wicri:doubleKey">0013-936X:2014:Bianchi F:insight:into:acid</idno><idno type="wicri:Area/Main/Merge">005634</idno><idno type="wicri:Area/Main/Curation">005349</idno><idno type="wicri:Area/Main/Exploration">005349</idno><idno type="wicri:Area/France/Extraction">000325</idno></publicationStmt><sourceDesc><biblStruct><analytic><title xml:lang="en" level="a">Insight into Acid-Base Nucleation Experiments by Comparison of the Chemical Composition of Positive, Negative, and Neutral Clusters</title><author><name sortKey="Bianchi, Federico" sort="Bianchi, Federico" uniqKey="Bianchi F" first="Federico" last="Bianchi">Federico Bianchi</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Laboratory of Atmospheric Chemistry, Paul Scherrer Institute</s1><s2>Villigen 5232</s2><s3>CHE</s3><sZ>1 aut.</sZ><sZ>4 aut.</sZ><sZ>10 aut.</sZ><sZ>28 aut.</sZ><sZ>36 aut.</sZ><sZ>40 aut.</sZ><sZ>50 aut.</sZ></inist:fA14><country>Suisse</country><wicri:noRegion>Villigen 5232</wicri:noRegion></affiliation></author><author><name sortKey="Praplan, Arnaud P" sort="Praplan, Arnaud P" uniqKey="Praplan A" first="Arnaud P." last="Praplan">Arnaud P. Praplan</name><affiliation wicri:level="4"><inist:fA14 i1="02"><s1>Departrnent of Physics, University of Helsinki</s1><s2>Helsinki 00014</s2><s3>FIN</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>7 aut.</sZ><sZ>8 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>17 aut.</sZ><sZ>20 aut.</sZ><sZ>21 aut.</sZ><sZ>24 aut.</sZ><sZ>30 aut.</sZ><sZ>35 aut.</sZ><sZ>37 aut.</sZ><sZ>43 aut.</sZ><sZ>47 aut.</sZ><sZ>48 aut.</sZ></inist:fA14><country>Finlande</country><placeName><settlement type="city">Helsinki</settlement><region type="région" nuts="2">Uusimaa</region></placeName><orgName type="university">Université d'Helsinki</orgName></affiliation></author><author><name sortKey="Sarnela, Nina" sort="Sarnela, Nina" uniqKey="Sarnela N" first="Nina" last="Sarnela">Nina Sarnela</name><affiliation wicri:level="4"><inist:fA14 i1="02"><s1>Departrnent of Physics, University of Helsinki</s1><s2>Helsinki 00014</s2><s3>FIN</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>7 aut.</sZ><sZ>8 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>17 aut.</sZ><sZ>20 aut.</sZ><sZ>21 aut.</sZ><sZ>24 aut.</sZ><sZ>30 aut.</sZ><sZ>35 aut.</sZ><sZ>37 aut.</sZ><sZ>43 aut.</sZ><sZ>47 aut.</sZ><sZ>48 aut.</sZ></inist:fA14><country>Finlande</country><placeName><settlement type="city">Helsinki</settlement><region type="région" nuts="2">Uusimaa</region></placeName><orgName type="university">Université d'Helsinki</orgName></affiliation></author><author><name sortKey="Dommen, Josef" sort="Dommen, Josef" uniqKey="Dommen J" first="Josef" last="Dommen">Josef Dommen</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Laboratory of Atmospheric Chemistry, Paul Scherrer Institute</s1><s2>Villigen 5232</s2><s3>CHE</s3><sZ>1 aut.</sZ><sZ>4 aut.</sZ><sZ>10 aut.</sZ><sZ>28 aut.</sZ><sZ>36 aut.</sZ><sZ>40 aut.</sZ><sZ>50 aut.</sZ></inist:fA14><country>Suisse</country><wicri:noRegion>Villigen 5232</wicri:noRegion></affiliation></author><author><name sortKey="Kurten, Andreas" sort="Kurten, Andreas" uniqKey="Kurten A" first="Andreas" last="Kürten">Andreas Kürten</name><affiliation wicri:level="3"><inist:fA14 i1="03"><s1>Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt am Main</s1><s2>Frankfurt am Main 60438</s2><s3>DEU</s3><sZ>5 aut.</sZ><sZ>9 aut.</sZ><sZ>23 aut.</sZ><sZ>27 aut.</sZ><sZ>31 aut.</sZ><sZ>38 aut.</sZ><sZ>42 aut.</sZ><sZ>43 aut.</sZ><sZ>46 aut.</sZ></inist:fA14><country>Allemagne</country><placeName><region type="land" nuts="1">Hesse (Land)</region><region type="district" nuts="2">District de Darmstadt</region><settlement type="city">Francfort-sur-le-Main</settlement></placeName></affiliation></author><author><name sortKey="Ortega, Ismael K" sort="Ortega, Ismael K" uniqKey="Ortega I" first="Ismael K." last="Ortega">Ismael K. Ortega</name><affiliation wicri:level="1"><inist:fA14 i1="04"><s1>Laboratoire de Physique des Lasers, Atomes et Molécules, Université Lille 1 Sciences et Technologies</s1><s2>Viileneuve d'Ascq 59655</s2><s3>FRA</s3><sZ>6 aut.</sZ></inist:fA14><country>France</country><wicri:noRegion>59655</wicri:noRegion><wicri:noRegion>Université Lille 1 Sciences et Technologies</wicri:noRegion><wicri:noRegion>Viileneuve d'Ascq 59655</wicri:noRegion></affiliation></author><author><name sortKey="Schobesberger, Siegfried" sort="Schobesberger, Siegfried" uniqKey="Schobesberger S" first="Siegfried" last="Schobesberger">Siegfried Schobesberger</name><affiliation wicri:level="4"><inist:fA14 i1="02"><s1>Departrnent of Physics, University of Helsinki</s1><s2>Helsinki 00014</s2><s3>FIN</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>7 aut.</sZ><sZ>8 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>17 aut.</sZ><sZ>20 aut.</sZ><sZ>21 aut.</sZ><sZ>24 aut.</sZ><sZ>30 aut.</sZ><sZ>35 aut.</sZ><sZ>37 aut.</sZ><sZ>43 aut.</sZ><sZ>47 aut.</sZ><sZ>48 aut.</sZ></inist:fA14><country>Finlande</country><placeName><settlement type="city">Helsinki</settlement><region type="région" nuts="2">Uusimaa</region></placeName><orgName type="university">Université d'Helsinki</orgName></affiliation></author><author><name sortKey="Junninen, Heikki" sort="Junninen, Heikki" uniqKey="Junninen H" first="Heikki" last="Junninen">Heikki Junninen</name><affiliation wicri:level="4"><inist:fA14 i1="02"><s1>Departrnent of Physics, University of Helsinki</s1><s2>Helsinki 00014</s2><s3>FIN</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>7 aut.</sZ><sZ>8 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>17 aut.</sZ><sZ>20 aut.</sZ><sZ>21 aut.</sZ><sZ>24 aut.</sZ><sZ>30 aut.</sZ><sZ>35 aut.</sZ><sZ>37 aut.</sZ><sZ>43 aut.</sZ><sZ>47 aut.</sZ><sZ>48 aut.</sZ></inist:fA14><country>Finlande</country><placeName><settlement type="city">Helsinki</settlement><region type="région" nuts="2">Uusimaa</region></placeName><orgName type="university">Université d'Helsinki</orgName></affiliation></author><author><name sortKey="Simon, Mario" sort="Simon, Mario" uniqKey="Simon M" first="Mario" last="Simon">Mario Simon</name><affiliation wicri:level="3"><inist:fA14 i1="03"><s1>Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt am Main</s1><s2>Frankfurt am Main 60438</s2><s3>DEU</s3><sZ>5 aut.</sZ><sZ>9 aut.</sZ><sZ>23 aut.</sZ><sZ>27 aut.</sZ><sZ>31 aut.</sZ><sZ>38 aut.</sZ><sZ>42 aut.</sZ><sZ>43 aut.</sZ><sZ>46 aut.</sZ></inist:fA14><country>Allemagne</country><placeName><region type="land" nuts="1">Hesse (Land)</region><region type="district" nuts="2">District de Darmstadt</region><settlement type="city">Francfort-sur-le-Main</settlement></placeName></affiliation></author><author><name sortKey="Trostl, Jasmin" sort="Trostl, Jasmin" uniqKey="Trostl J" first="Jasmin" last="Tröstl">Jasmin Tröstl</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Laboratory of Atmospheric Chemistry, Paul Scherrer Institute</s1><s2>Villigen 5232</s2><s3>CHE</s3><sZ>1 aut.</sZ><sZ>4 aut.</sZ><sZ>10 aut.</sZ><sZ>28 aut.</sZ><sZ>36 aut.</sZ><sZ>40 aut.</sZ><sZ>50 aut.</sZ></inist:fA14><country>Suisse</country><wicri:noRegion>Villigen 5232</wicri:noRegion></affiliation></author><author><name sortKey="Jokinen, Tuija" sort="Jokinen, Tuija" uniqKey="Jokinen T" first="Tuija" last="Jokinen">Tuija Jokinen</name><affiliation wicri:level="4"><inist:fA14 i1="02"><s1>Departrnent of Physics, University of Helsinki</s1><s2>Helsinki 00014</s2><s3>FIN</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>7 aut.</sZ><sZ>8 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>17 aut.</sZ><sZ>20 aut.</sZ><sZ>21 aut.</sZ><sZ>24 aut.</sZ><sZ>30 aut.</sZ><sZ>35 aut.</sZ><sZ>37 aut.</sZ><sZ>43 aut.</sZ><sZ>47 aut.</sZ><sZ>48 aut.</sZ></inist:fA14><country>Finlande</country><placeName><settlement type="city">Helsinki</settlement><region type="région" nuts="2">Uusimaa</region></placeName><orgName type="university">Université d'Helsinki</orgName></affiliation></author><author><name sortKey="Sipil, Mikko" sort="Sipil, Mikko" uniqKey="Sipil M" first="Mikko" last="Sipil">Mikko Sipil</name><affiliation wicri:level="4"><inist:fA14 i1="02"><s1>Departrnent of Physics, University of Helsinki</s1><s2>Helsinki 00014</s2><s3>FIN</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>7 aut.</sZ><sZ>8 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>17 aut.</sZ><sZ>20 aut.</sZ><sZ>21 aut.</sZ><sZ>24 aut.</sZ><sZ>30 aut.</sZ><sZ>35 aut.</sZ><sZ>37 aut.</sZ><sZ>43 aut.</sZ><sZ>47 aut.</sZ><sZ>48 aut.</sZ></inist:fA14><country>Finlande</country><placeName><settlement type="city">Helsinki</settlement><region type="région" nuts="2">Uusimaa</region></placeName><orgName type="university">Université d'Helsinki</orgName></affiliation></author><author><name sortKey="Adamov, Alexey" sort="Adamov, Alexey" uniqKey="Adamov A" first="Alexey" last="Adamov">Alexey Adamov</name><affiliation wicri:level="4"><inist:fA14 i1="02"><s1>Departrnent of Physics, University of Helsinki</s1><s2>Helsinki 00014</s2><s3>FIN</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>7 aut.</sZ><sZ>8 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>17 aut.</sZ><sZ>20 aut.</sZ><sZ>21 aut.</sZ><sZ>24 aut.</sZ><sZ>30 aut.</sZ><sZ>35 aut.</sZ><sZ>37 aut.</sZ><sZ>43 aut.</sZ><sZ>47 aut.</sZ><sZ>48 aut.</sZ></inist:fA14><country>Finlande</country><placeName><settlement type="city">Helsinki</settlement><region type="région" nuts="2">Uusimaa</region></placeName><orgName type="university">Université d'Helsinki</orgName></affiliation></author><author><name sortKey="Amonm, Antonio" sort="Amonm, Antonio" uniqKey="Amonm A" first="Antonio" last="Amonm">Antonio Amonm</name><affiliation wicri:level="1"><inist:fA14 i1="05"><s1>CENTRA-SIM, U. Lisboa and U. Beira Interior</s1><s2>Lisbon 1749</s2><s3>PRT</s3><sZ>14 aut.</sZ><sZ>39 aut.</sZ></inist:fA14><country>Portugal</country><wicri:noRegion>Lisbon 1749</wicri:noRegion></affiliation></author><author><name sortKey="Almeida, Joao" sort="Almeida, Joao" uniqKey="Almeida J" first="Joao" last="Almeida">Joao Almeida</name><affiliation wicri:level="1"><inist:fA14 i1="06"><s1>CERN</s1><s2>Geneva 1211</s2><s3>CHE</s3><sZ>15 aut.</sZ><sZ>17 aut.</sZ><sZ>18 aut.</sZ><sZ>27 aut.</sZ><sZ>33 aut.</sZ><sZ>34 aut.</sZ></inist:fA14><country>Suisse</country><wicri:noRegion>CERN</wicri:noRegion></affiliation></author><author><name sortKey="Breitenlechner, Martin" sort="Breitenlechner, Martin" uniqKey="Breitenlechner M" first="Martin" last="Breitenlechner">Martin Breitenlechner</name><affiliation wicri:level="1"><inist:fA14 i1="07"><s1>University of Innsbruck</s1><s2>Innsbruck 6020</s2><s3>AUT</s3><sZ>16 aut.</sZ><sZ>22 aut.</sZ><sZ>23 aut.</sZ></inist:fA14><country>Autriche</country><wicri:noRegion>University of Innsbruck</wicri:noRegion></affiliation><affiliation wicri:level="1"><inist:fA14 i1="08"><s1>IONICON Analytik GmbH</s1><s2>Innsbruck 6020</s2><s3>AUT</s3><sZ>16 aut.</sZ><sZ>22 aut.</sZ></inist:fA14><country>Autriche</country><wicri:noRegion>IONICON Analytik GmbH</wicri:noRegion></affiliation></author><author><name sortKey="Duplissy, Jonathan" sort="Duplissy, Jonathan" uniqKey="Duplissy J" first="Jonathan" last="Duplissy">Jonathan Duplissy</name><affiliation wicri:level="4"><inist:fA14 i1="02"><s1>Departrnent of Physics, University of Helsinki</s1><s2>Helsinki 00014</s2><s3>FIN</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>7 aut.</sZ><sZ>8 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>17 aut.</sZ><sZ>20 aut.</sZ><sZ>21 aut.</sZ><sZ>24 aut.</sZ><sZ>30 aut.</sZ><sZ>35 aut.</sZ><sZ>37 aut.</sZ><sZ>43 aut.</sZ><sZ>47 aut.</sZ><sZ>48 aut.</sZ></inist:fA14><country>Finlande</country><placeName><settlement type="city">Helsinki</settlement><region type="région" nuts="2">Uusimaa</region></placeName><orgName type="university">Université d'Helsinki</orgName></affiliation><affiliation wicri:level="1"><inist:fA14 i1="06"><s1>CERN</s1><s2>Geneva 1211</s2><s3>CHE</s3><sZ>15 aut.</sZ><sZ>17 aut.</sZ><sZ>18 aut.</sZ><sZ>27 aut.</sZ><sZ>33 aut.</sZ><sZ>34 aut.</sZ></inist:fA14><country>Suisse</country><wicri:noRegion>CERN</wicri:noRegion></affiliation><affiliation wicri:level="1"><inist:fA14 i1="09"><s1>Helsinki Institute of Physics</s1><s2>Helsinki 00014</s2><s3>FIN</s3><sZ>17 aut.</sZ></inist:fA14><country>Finlande</country><wicri:noRegion>Helsinki Institute of Physics</wicri:noRegion></affiliation></author><author><name sortKey="Ehrhart, Sebastian" sort="Ehrhart, Sebastian" uniqKey="Ehrhart S" first="Sebastian" last="Ehrhart">Sebastian Ehrhart</name><affiliation wicri:level="1"><inist:fA14 i1="06"><s1>CERN</s1><s2>Geneva 1211</s2><s3>CHE</s3><sZ>15 aut.</sZ><sZ>17 aut.</sZ><sZ>18 aut.</sZ><sZ>27 aut.</sZ><sZ>33 aut.</sZ><sZ>34 aut.</sZ></inist:fA14><country>Suisse</country><wicri:noRegion>CERN</wicri:noRegion></affiliation></author><author><name sortKey="Flagan, Richard C" sort="Flagan, Richard C" uniqKey="Flagan R" first="Richard C." last="Flagan">Richard C. Flagan</name><affiliation wicri:level="1"><inist:fA14 i1="10"><s1>Califomia Institute of Technology</s1><s2>Pasadena, California 91125</s2><s3>USA</s3><sZ>19 aut.</sZ></inist:fA14><country>États-Unis</country><wicri:noRegion>Califomia Institute of Technology</wicri:noRegion></affiliation></author><author><name sortKey="Franchin, Alessandro" sort="Franchin, Alessandro" uniqKey="Franchin A" first="Alessandro" last="Franchin">Alessandro Franchin</name><affiliation wicri:level="4"><inist:fA14 i1="02"><s1>Departrnent of Physics, University of Helsinki</s1><s2>Helsinki 00014</s2><s3>FIN</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>7 aut.</sZ><sZ>8 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>17 aut.</sZ><sZ>20 aut.</sZ><sZ>21 aut.</sZ><sZ>24 aut.</sZ><sZ>30 aut.</sZ><sZ>35 aut.</sZ><sZ>37 aut.</sZ><sZ>43 aut.</sZ><sZ>47 aut.</sZ><sZ>48 aut.</sZ></inist:fA14><country>Finlande</country><placeName><settlement type="city">Helsinki</settlement><region type="région" nuts="2">Uusimaa</region></placeName><orgName type="university">Université d'Helsinki</orgName></affiliation></author><author><name sortKey="Hakala, Jani" sort="Hakala, Jani" uniqKey="Hakala J" first="Jani" last="Hakala">Jani Hakala</name><affiliation wicri:level="4"><inist:fA14 i1="02"><s1>Departrnent of Physics, University of Helsinki</s1><s2>Helsinki 00014</s2><s3>FIN</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>7 aut.</sZ><sZ>8 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>17 aut.</sZ><sZ>20 aut.</sZ><sZ>21 aut.</sZ><sZ>24 aut.</sZ><sZ>30 aut.</sZ><sZ>35 aut.</sZ><sZ>37 aut.</sZ><sZ>43 aut.</sZ><sZ>47 aut.</sZ><sZ>48 aut.</sZ></inist:fA14><country>Finlande</country><placeName><settlement type="city">Helsinki</settlement><region type="région" nuts="2">Uusimaa</region></placeName><orgName type="university">Université d'Helsinki</orgName></affiliation></author><author><name sortKey="Hansel, Armin" sort="Hansel, Armin" uniqKey="Hansel A" first="Armin" last="Hansel">Armin Hansel</name><affiliation wicri:level="1"><inist:fA14 i1="07"><s1>University of Innsbruck</s1><s2>Innsbruck 6020</s2><s3>AUT</s3><sZ>16 aut.</sZ><sZ>22 aut.</sZ><sZ>23 aut.</sZ></inist:fA14><country>Autriche</country><wicri:noRegion>University of Innsbruck</wicri:noRegion></affiliation><affiliation wicri:level="1"><inist:fA14 i1="08"><s1>IONICON Analytik GmbH</s1><s2>Innsbruck 6020</s2><s3>AUT</s3><sZ>16 aut.</sZ><sZ>22 aut.</sZ></inist:fA14><country>Autriche</country><wicri:noRegion>IONICON Analytik GmbH</wicri:noRegion></affiliation></author><author><name sortKey="Heinritzi, Martin" sort="Heinritzi, Martin" uniqKey="Heinritzi M" first="Martin" last="Heinritzi">Martin Heinritzi</name><affiliation wicri:level="3"><inist:fA14 i1="03"><s1>Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt am Main</s1><s2>Frankfurt am Main 60438</s2><s3>DEU</s3><sZ>5 aut.</sZ><sZ>9 aut.</sZ><sZ>23 aut.</sZ><sZ>27 aut.</sZ><sZ>31 aut.</sZ><sZ>38 aut.</sZ><sZ>42 aut.</sZ><sZ>43 aut.</sZ><sZ>46 aut.</sZ></inist:fA14><country>Allemagne</country><placeName><region type="land" nuts="1">Hesse (Land)</region><region type="district" nuts="2">District de Darmstadt</region><settlement type="city">Francfort-sur-le-Main</settlement></placeName></affiliation><affiliation wicri:level="1"><inist:fA14 i1="07"><s1>University of Innsbruck</s1><s2>Innsbruck 6020</s2><s3>AUT</s3><sZ>16 aut.</sZ><sZ>22 aut.</sZ><sZ>23 aut.</sZ></inist:fA14><country>Autriche</country><wicri:noRegion>University of Innsbruck</wicri:noRegion></affiliation></author><author><name sortKey="Kangasluoma, Juha" sort="Kangasluoma, Juha" uniqKey="Kangasluoma J" first="Juha" last="Kangasluoma">Juha Kangasluoma</name><affiliation wicri:level="4"><inist:fA14 i1="02"><s1>Departrnent of Physics, University of Helsinki</s1><s2>Helsinki 00014</s2><s3>FIN</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>7 aut.</sZ><sZ>8 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>17 aut.</sZ><sZ>20 aut.</sZ><sZ>21 aut.</sZ><sZ>24 aut.</sZ><sZ>30 aut.</sZ><sZ>35 aut.</sZ><sZ>37 aut.</sZ><sZ>43 aut.</sZ><sZ>47 aut.</sZ><sZ>48 aut.</sZ></inist:fA14><country>Finlande</country><placeName><settlement type="city">Helsinki</settlement><region type="région" nuts="2">Uusimaa</region></placeName><orgName type="university">Université d'Helsinki</orgName></affiliation></author><author><name sortKey="Keskinen, Helmi" sort="Keskinen, Helmi" uniqKey="Keskinen H" first="Helmi" last="Keskinen">Helmi Keskinen</name><affiliation wicri:level="1"><inist:fA14 i1="11"><s1>Department of Applied Physics, University of Eastern Finland</s1><s2>Kuopio 70211</s2><s3>FIN</s3><sZ>25 aut.</sZ><sZ>26 aut.</sZ><sZ>29 aut.</sZ></inist:fA14><country>Finlande</country><wicri:noRegion>Kuopio 70211</wicri:noRegion></affiliation></author><author><name sortKey="Jaeseok Kim" sort="Jaeseok Kim" uniqKey="Jaeseok Kim" last="Jaeseok Kim">JAESEOK KIM</name><affiliation wicri:level="1"><inist:fA14 i1="11"><s1>Department of Applied Physics, University of Eastern Finland</s1><s2>Kuopio 70211</s2><s3>FIN</s3><sZ>25 aut.</sZ><sZ>26 aut.</sZ><sZ>29 aut.</sZ></inist:fA14><country>Finlande</country><wicri:noRegion>Kuopio 70211</wicri:noRegion></affiliation></author><author><name sortKey="Kirkby, Jasper" sort="Kirkby, Jasper" uniqKey="Kirkby J" first="Jasper" last="Kirkby">Jasper Kirkby</name><affiliation wicri:level="3"><inist:fA14 i1="03"><s1>Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt am Main</s1><s2>Frankfurt am Main 60438</s2><s3>DEU</s3><sZ>5 aut.</sZ><sZ>9 aut.</sZ><sZ>23 aut.</sZ><sZ>27 aut.</sZ><sZ>31 aut.</sZ><sZ>38 aut.</sZ><sZ>42 aut.</sZ><sZ>43 aut.</sZ><sZ>46 aut.</sZ></inist:fA14><country>Allemagne</country><placeName><region type="land" nuts="1">Hesse (Land)</region><region type="district" nuts="2">District de Darmstadt</region><settlement type="city">Francfort-sur-le-Main</settlement></placeName></affiliation><affiliation wicri:level="1"><inist:fA14 i1="06"><s1>CERN</s1><s2>Geneva 1211</s2><s3>CHE</s3><sZ>15 aut.</sZ><sZ>17 aut.</sZ><sZ>18 aut.</sZ><sZ>27 aut.</sZ><sZ>33 aut.</sZ><sZ>34 aut.</sZ></inist:fA14><country>Suisse</country><wicri:noRegion>CERN</wicri:noRegion></affiliation></author><author><name sortKey="Laaksonen, Ari" sort="Laaksonen, Ari" uniqKey="Laaksonen A" first="Ari" last="Laaksonen">Ari Laaksonen</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Laboratory of Atmospheric Chemistry, Paul Scherrer Institute</s1><s2>Villigen 5232</s2><s3>CHE</s3><sZ>1 aut.</sZ><sZ>4 aut.</sZ><sZ>10 aut.</sZ><sZ>28 aut.</sZ><sZ>36 aut.</sZ><sZ>40 aut.</sZ><sZ>50 aut.</sZ></inist:fA14><country>Suisse</country><wicri:noRegion>Villigen 5232</wicri:noRegion></affiliation><affiliation wicri:level="1"><inist:fA14 i1="15"><s1>Finnish Meteorological Institute</s1><s2>Helsinki 00101</s2><s3>FIN</s3><sZ>28 aut.</sZ><sZ>41 aut.</sZ></inist:fA14><country>Finlande</country><wicri:noRegion>Finnish Meteorological Institute</wicri:noRegion></affiliation></author><author><name sortKey="Lawler, Michael J" sort="Lawler, Michael J" uniqKey="Lawler M" first="Michael J." last="Lawler">Michael J. Lawler</name><affiliation wicri:level="1"><inist:fA14 i1="11"><s1>Department of Applied Physics, University of Eastern Finland</s1><s2>Kuopio 70211</s2><s3>FIN</s3><sZ>25 aut.</sZ><sZ>26 aut.</sZ><sZ>29 aut.</sZ></inist:fA14><country>Finlande</country><wicri:noRegion>Kuopio 70211</wicri:noRegion></affiliation><affiliation wicri:level="1"><inist:fA14 i1="12"><s1>Atmospheric Chemistry Division, National Center for Atmospheric Research</s1><s2>Boulder, Colorado 80301</s2><s3>USA</s3><sZ>29 aut.</sZ></inist:fA14><country>États-Unis</country><wicri:noRegion>Boulder, Colorado 80301</wicri:noRegion></affiliation></author><author><name sortKey="Lehtipalo, Katrianne" sort="Lehtipalo, Katrianne" uniqKey="Lehtipalo K" first="Katrianne" last="Lehtipalo">Katrianne Lehtipalo</name><affiliation wicri:level="4"><inist:fA14 i1="02"><s1>Departrnent of Physics, University of Helsinki</s1><s2>Helsinki 00014</s2><s3>FIN</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>7 aut.</sZ><sZ>8 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>17 aut.</sZ><sZ>20 aut.</sZ><sZ>21 aut.</sZ><sZ>24 aut.</sZ><sZ>30 aut.</sZ><sZ>35 aut.</sZ><sZ>37 aut.</sZ><sZ>43 aut.</sZ><sZ>47 aut.</sZ><sZ>48 aut.</sZ></inist:fA14><country>Finlande</country><placeName><settlement type="city">Helsinki</settlement><region type="région" nuts="2">Uusimaa</region></placeName><orgName type="university">Université d'Helsinki</orgName></affiliation><affiliation wicri:level="1"><inist:fA14 i1="13"><s1>Airmodus Ltd</s1><s2>Helsinki 00560</s2><s3>FIN</s3><sZ>30 aut.</sZ></inist:fA14><country>Finlande</country><wicri:noRegion>Airmodus Ltd</wicri:noRegion></affiliation></author><author><name sortKey="Leiminger, Markus" sort="Leiminger, Markus" uniqKey="Leiminger M" first="Markus" last="Leiminger">Markus Leiminger</name><affiliation wicri:level="3"><inist:fA14 i1="03"><s1>Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt am Main</s1><s2>Frankfurt am Main 60438</s2><s3>DEU</s3><sZ>5 aut.</sZ><sZ>9 aut.</sZ><sZ>23 aut.</sZ><sZ>27 aut.</sZ><sZ>31 aut.</sZ><sZ>38 aut.</sZ><sZ>42 aut.</sZ><sZ>43 aut.</sZ><sZ>46 aut.</sZ></inist:fA14><country>Allemagne</country><placeName><region type="land" nuts="1">Hesse (Land)</region><region type="district" nuts="2">District de Darmstadt</region><settlement type="city">Francfort-sur-le-Main</settlement></placeName></affiliation></author><author><name sortKey="Makhmutov, Vladimir" sort="Makhmutov, Vladimir" uniqKey="Makhmutov V" first="Vladimir" last="Makhmutov">Vladimir Makhmutov</name><affiliation wicri:level="1"><inist:fA14 i1="14"><s1>Lebedev Physical Institute RAS, Leninsky prospekt</s1><s2>Moscow 119991</s2><s3>RUS</s3><sZ>32 aut.</sZ></inist:fA14><country>Russie</country><placeName><settlement type="city">Moscou</settlement><region>District fédéral central</region></placeName></affiliation></author><author><name sortKey="Mathot, Serge" sort="Mathot, Serge" uniqKey="Mathot S" first="Serge" last="Mathot">Serge Mathot</name><affiliation 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aut.</sZ><sZ>8 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>17 aut.</sZ><sZ>20 aut.</sZ><sZ>21 aut.</sZ><sZ>24 aut.</sZ><sZ>30 aut.</sZ><sZ>35 aut.</sZ><sZ>37 aut.</sZ><sZ>43 aut.</sZ><sZ>47 aut.</sZ><sZ>48 aut.</sZ></inist:fA14><country>Finlande</country><placeName><settlement type="city">Helsinki</settlement><region type="région" nuts="2">Uusimaa</region></placeName><orgName type="university">Université d'Helsinki</orgName></affiliation></author><author><name sortKey="Riccobono, Francesco" sort="Riccobono, Francesco" uniqKey="Riccobono F" first="Francesco" last="Riccobono">Francesco Riccobono</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Laboratory of Atmospheric Chemistry, Paul Scherrer Institute</s1><s2>Villigen 5232</s2><s3>CHE</s3><sZ>1 aut.</sZ><sZ>4 aut.</sZ><sZ>10 aut.</sZ><sZ>28 aut.</sZ><sZ>36 aut.</sZ><sZ>40 aut.</sZ><sZ>50 aut.</sZ></inist:fA14><country>Suisse</country><wicri:noRegion>Villigen 5232</wicri:noRegion></affiliation></author><author><name sortKey="Rissanen, Matti P" sort="Rissanen, Matti P" uniqKey="Rissanen M" first="Matti P." last="Rissanen">Matti P. Rissanen</name><affiliation wicri:level="4"><inist:fA14 i1="02"><s1>Departrnent of Physics, University of Helsinki</s1><s2>Helsinki 00014</s2><s3>FIN</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>7 aut.</sZ><sZ>8 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>17 aut.</sZ><sZ>20 aut.</sZ><sZ>21 aut.</sZ><sZ>24 aut.</sZ><sZ>30 aut.</sZ><sZ>35 aut.</sZ><sZ>37 aut.</sZ><sZ>43 aut.</sZ><sZ>47 aut.</sZ><sZ>48 aut.</sZ></inist:fA14><country>Finlande</country><placeName><settlement type="city">Helsinki</settlement><region type="région" nuts="2">Uusimaa</region></placeName><orgName type="university">Université d'Helsinki</orgName></affiliation></author><author><name sortKey="Rondo, Linda" sort="Rondo, Linda" uniqKey="Rondo L" first="Linda" last="Rondo">Linda Rondo</name><affiliation wicri:level="3"><inist:fA14 i1="03"><s1>Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt am Main</s1><s2>Frankfurt am Main 60438</s2><s3>DEU</s3><sZ>5 aut.</sZ><sZ>9 aut.</sZ><sZ>23 aut.</sZ><sZ>27 aut.</sZ><sZ>31 aut.</sZ><sZ>38 aut.</sZ><sZ>42 aut.</sZ><sZ>43 aut.</sZ><sZ>46 aut.</sZ></inist:fA14><country>Allemagne</country><placeName><region type="land" nuts="1">Hesse (Land)</region><region type="district" nuts="2">District de Darmstadt</region><settlement type="city">Francfort-sur-le-Main</settlement></placeName></affiliation></author><author><name sortKey="Tome, Ant Nio" sort="Tome, Ant Nio" uniqKey="Tome A" first="Ant Nio" last="Tome">Ant Nio Tome</name><affiliation wicri:level="1"><inist:fA14 i1="05"><s1>CENTRA-SIM, U. Lisboa and U. Beira Interior</s1><s2>Lisbon 1749</s2><s3>PRT</s3><sZ>14 aut.</sZ><sZ>39 aut.</sZ></inist:fA14><country>Portugal</country><wicri:noRegion>Lisbon 1749</wicri:noRegion></affiliation></author><author><name sortKey="Virtanen, Annele" sort="Virtanen, Annele" uniqKey="Virtanen A" first="Annele" last="Virtanen">Annele Virtanen</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Laboratory of Atmospheric Chemistry, Paul Scherrer Institute</s1><s2>Villigen 5232</s2><s3>CHE</s3><sZ>1 aut.</sZ><sZ>4 aut.</sZ><sZ>10 aut.</sZ><sZ>28 aut.</sZ><sZ>36 aut.</sZ><sZ>40 aut.</sZ><sZ>50 aut.</sZ></inist:fA14><country>Suisse</country><wicri:noRegion>Villigen 5232</wicri:noRegion></affiliation></author><author><name sortKey="Viisanen, Yrjo" sort="Viisanen, Yrjo" uniqKey="Viisanen Y" first="Yrjö" last="Viisanen">Yrjö Viisanen</name><affiliation wicri:level="1"><inist:fA14 i1="15"><s1>Finnish Meteorological Institute</s1><s2>Helsinki 00101</s2><s3>FIN</s3><sZ>28 aut.</sZ><sZ>41 aut.</sZ></inist:fA14><country>Finlande</country><wicri:noRegion>Finnish Meteorological Institute</wicri:noRegion></affiliation></author><author><name sortKey="Williamson, Christina" sort="Williamson, Christina" uniqKey="Williamson C" first="Christina" last="Williamson">Christina Williamson</name><affiliation wicri:level="3"><inist:fA14 i1="03"><s1>Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt am Main</s1><s2>Frankfurt am Main 60438</s2><s3>DEU</s3><sZ>5 aut.</sZ><sZ>9 aut.</sZ><sZ>23 aut.</sZ><sZ>27 aut.</sZ><sZ>31 aut.</sZ><sZ>38 aut.</sZ><sZ>42 aut.</sZ><sZ>43 aut.</sZ><sZ>46 aut.</sZ></inist:fA14><country>Allemagne</country><placeName><region type="land" nuts="1">Hesse (Land)</region><region type="district" nuts="2">District de Darmstadt</region><settlement type="city">Francfort-sur-le-Main</settlement></placeName></affiliation></author><author><name sortKey="Wimmer, Daniela" sort="Wimmer, Daniela" uniqKey="Wimmer D" first="Daniela" last="Wimmer">Daniela Wimmer</name><affiliation wicri:level="4"><inist:fA14 i1="02"><s1>Departrnent of Physics, University of Helsinki</s1><s2>Helsinki 00014</s2><s3>FIN</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>7 aut.</sZ><sZ>8 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>17 aut.</sZ><sZ>20 aut.</sZ><sZ>21 aut.</sZ><sZ>24 aut.</sZ><sZ>30 aut.</sZ><sZ>35 aut.</sZ><sZ>37 aut.</sZ><sZ>43 aut.</sZ><sZ>47 aut.</sZ><sZ>48 aut.</sZ></inist:fA14><country>Finlande</country><placeName><settlement type="city">Helsinki</settlement><region type="région" nuts="2">Uusimaa</region></placeName><orgName type="university">Université d'Helsinki</orgName></affiliation><affiliation wicri:level="3"><inist:fA14 i1="03"><s1>Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt am Main</s1><s2>Frankfurt am Main 60438</s2><s3>DEU</s3><sZ>5 aut.</sZ><sZ>9 aut.</sZ><sZ>23 aut.</sZ><sZ>27 aut.</sZ><sZ>31 aut.</sZ><sZ>38 aut.</sZ><sZ>42 aut.</sZ><sZ>43 aut.</sZ><sZ>46 aut.</sZ></inist:fA14><country>Allemagne</country><placeName><region type="land" nuts="1">Hesse (Land)</region><region type="district" nuts="2">District de Darmstadt</region><settlement type="city">Francfort-sur-le-Main</settlement></placeName></affiliation></author><author><name sortKey="Winkler, Paul M" sort="Winkler, Paul M" uniqKey="Winkler P" first="Paul M." last="Winkler">Paul M. Winkler</name><affiliation wicri:level="1"><inist:fA14 i1="16"><s1>Faculty of Physics, University of Vienna</s1><s2>Vienna 1090</s2><s3>AUT</s3><sZ>44 aut.</sZ></inist:fA14><country>Autriche</country><placeName><settlement type="city">Vienne (Autriche)</settlement><region nuts="2" type="province">Vienne (Autriche)</region></placeName></affiliation></author><author><name sortKey="Penglin Ye" sort="Penglin Ye" uniqKey="Penglin Ye" last="Penglin Ye">PENGLIN YE</name><affiliation wicri:level="4"><inist:fA14 i1="17"><s1>Center for Atmospheric Particle Studies, Carnegie Mellon University</s1><s2>Pittsburgh, Pennsylvania 15213</s2><s3>USA</s3><sZ>45 aut.</sZ><sZ>49 aut.</sZ></inist:fA14><country>États-Unis</country><placeName><settlement type="city">Pittsburgh</settlement><region type="state">Pennsylvanie</region></placeName><orgName type="university">Université Carnegie-Mellon</orgName></affiliation></author><author><name sortKey="Curtius, Joachim" sort="Curtius, Joachim" uniqKey="Curtius J" first="Joachim" last="Curtius">Joachim Curtius</name><affiliation wicri:level="3"><inist:fA14 i1="03"><s1>Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt am Main</s1><s2>Frankfurt am Main 60438</s2><s3>DEU</s3><sZ>5 aut.</sZ><sZ>9 aut.</sZ><sZ>23 aut.</sZ><sZ>27 aut.</sZ><sZ>31 aut.</sZ><sZ>38 aut.</sZ><sZ>42 aut.</sZ><sZ>43 aut.</sZ><sZ>46 aut.</sZ></inist:fA14><country>Allemagne</country><placeName><region type="land" nuts="1">Hesse (Land)</region><region type="district" nuts="2">District de Darmstadt</region><settlement type="city">Francfort-sur-le-Main</settlement></placeName></affiliation></author><author><name sortKey="Kuimala, Markku" sort="Kuimala, Markku" uniqKey="Kuimala M" first="Markku" last="Kuimala">Markku Kuimala</name><affiliation wicri:level="4"><inist:fA14 i1="02"><s1>Departrnent of Physics, University of Helsinki</s1><s2>Helsinki 00014</s2><s3>FIN</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>7 aut.</sZ><sZ>8 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>17 aut.</sZ><sZ>20 aut.</sZ><sZ>21 aut.</sZ><sZ>24 aut.</sZ><sZ>30 aut.</sZ><sZ>35 aut.</sZ><sZ>37 aut.</sZ><sZ>43 aut.</sZ><sZ>47 aut.</sZ><sZ>48 aut.</sZ></inist:fA14><country>Finlande</country><placeName><settlement type="city">Helsinki</settlement><region type="région" nuts="2">Uusimaa</region></placeName><orgName type="university">Université d'Helsinki</orgName></affiliation></author><author><name sortKey="Worsnop, Douglas R" sort="Worsnop, Douglas R" uniqKey="Worsnop D" first="Douglas R." last="Worsnop">Douglas R. Worsnop</name><affiliation wicri:level="4"><inist:fA14 i1="02"><s1>Departrnent of Physics, University of Helsinki</s1><s2>Helsinki 00014</s2><s3>FIN</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>7 aut.</sZ><sZ>8 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>17 aut.</sZ><sZ>20 aut.</sZ><sZ>21 aut.</sZ><sZ>24 aut.</sZ><sZ>30 aut.</sZ><sZ>35 aut.</sZ><sZ>37 aut.</sZ><sZ>43 aut.</sZ><sZ>47 aut.</sZ><sZ>48 aut.</sZ></inist:fA14><country>Finlande</country><placeName><settlement type="city">Helsinki</settlement><region type="région" nuts="2">Uusimaa</region></placeName><orgName type="university">Université d'Helsinki</orgName></affiliation><affiliation wicri:level="1"><inist:fA14 i1="18"><s1>Aerodyne Research Inc.</s1><s2>Billerica, Massachusetts 01821</s2><s3>USA</s3><sZ>48 aut.</sZ></inist:fA14><country>États-Unis</country><wicri:noRegion>Aerodyne Research Inc.</wicri:noRegion></affiliation></author><author><name sortKey="Donahue, Neil M" sort="Donahue, Neil M" uniqKey="Donahue N" first="Neil M." last="Donahue">Neil M. Donahue</name><affiliation wicri:level="4"><inist:fA14 i1="17"><s1>Center for Atmospheric Particle Studies, Carnegie Mellon University</s1><s2>Pittsburgh, Pennsylvania 15213</s2><s3>USA</s3><sZ>45 aut.</sZ><sZ>49 aut.</sZ></inist:fA14><country>États-Unis</country><placeName><settlement type="city">Pittsburgh</settlement><region type="state">Pennsylvanie</region></placeName><orgName type="university">Université Carnegie-Mellon</orgName></affiliation></author><author><name sortKey="Baltensperger, Urs" sort="Baltensperger, Urs" uniqKey="Baltensperger U" first="Urs" last="Baltensperger">Urs Baltensperger</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Laboratory of Atmospheric Chemistry, Paul Scherrer Institute</s1><s2>Villigen 5232</s2><s3>CHE</s3><sZ>1 aut.</sZ><sZ>4 aut.</sZ><sZ>10 aut.</sZ><sZ>28 aut.</sZ><sZ>36 aut.</sZ><sZ>40 aut.</sZ><sZ>50 aut.</sZ></inist:fA14><country>Suisse</country><wicri:noRegion>Villigen 5232</wicri:noRegion></affiliation></author></analytic><series><title level="j" type="main">Environmental science & technology</title><title level="j" type="abbreviated">Environ. sci. technol.</title><idno type="ISSN">0013-936X</idno><imprint><date when="2014">2014</date></imprint></series></biblStruct></sourceDesc><seriesStmt><title level="j" type="main">Environmental science & technology</title><title level="j" type="abbreviated">Environ. sci. technol.</title><idno type="ISSN">0013-936X</idno></seriesStmt></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Air pollution</term><term>Amine</term><term>Atomic cluster</term><term>Ionic cluster</term><term>Laboratory study</term><term>Particle collision</term><term>Pollutant formation</term><term>Time of flight mass spectroscopy</term><term>aerosols</term><term>ammonia(compound)</term><term>nucleation</term><term>sulfuric acid</term></keywords><keywords scheme="Pascal" xml:lang="fr"><term>Etude en laboratoire</term><term>Aérosol</term><term>Nucléation</term><term>Acide sulfurique</term><term>Ammoniac</term><term>Amine</term><term>Agrégat ionique</term><term>Agrégat atomique</term><term>Spectrométrie masse temps vol</term><term>Collision particule</term><term>Pollution air</term><term>Formation polluant</term></keywords><keywords scheme="Wicri" type="topic" xml:lang="fr"><term>Aérosol</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">We investigated the nucleation of sulfuric acid together with two bases (ammonia and dimethylamine), at the CLOUD chamber at CERN. The chemical composition of positive, negative, and neutral clusters was studied using three Atmospheric Pressure interface-Time Of Flight (APi-TOF) mass spectrometers: two were operated in positive and negative mode to detect the chamber ions, while the third was equipped with a nitrate ion chemical ionization source allowing detection of neutral clusters. Taking into account the possible fragmentation that can happen during the charging of the ions or within the first stage of the mass spectrometer, the cluster formation proceeded via essentially one-to-one acid-base addition for all of the clusters, independent of the type of the base. For the positive clusters, the charge is carried by one excess protonated base, while for the negative clusters it is carried by a deprotonated add; the same is true for the neutral clusters after these have been ionized During the experiments involving sulfuric acid and dimethylamine, it was possible to study the appearance time for all the clusters (positive, negative, and neutral). It appeared that, after the formation of the clusters containing three molecules of sulfuric acid, the clusters grow at a similar speed, independent of their charge. The growth rate is then probably limited by the arrival rate of sulfuric acid or cluster-cluster collision.</div></front></TEI><affiliations><list><country><li>Allemagne</li><li>Autriche</li><li>Finlande</li><li>France</li><li>Portugal</li><li>Russie</li><li>Suisse</li><li>États-Unis</li></country><region><li>District de Darmstadt</li><li>District fédéral central</li><li>Hesse (Land)</li><li>Pennsylvanie</li><li>Uusimaa</li><li>Vienne (Autriche)</li></region><settlement><li>Francfort-sur-le-Main</li><li>Helsinki</li><li>Moscou</li><li>Pittsburgh</li><li>Vienne (Autriche)</li></settlement><orgName><li>Université Carnegie-Mellon</li><li>Université d'Helsinki</li></orgName></list><tree><country name="Suisse"><noRegion><name sortKey="Bianchi, Federico" sort="Bianchi, Federico" uniqKey="Bianchi F" first="Federico" last="Bianchi">Federico Bianchi</name></noRegion><name sortKey="Almeida, Joao" sort="Almeida, Joao" uniqKey="Almeida J" first="Joao" last="Almeida">Joao Almeida</name><name sortKey="Baltensperger, Urs" sort="Baltensperger, Urs" uniqKey="Baltensperger U" first="Urs" last="Baltensperger">Urs Baltensperger</name><name sortKey="Dommen, Josef" sort="Dommen, Josef" uniqKey="Dommen J" first="Josef" last="Dommen">Josef Dommen</name><name sortKey="Duplissy, Jonathan" sort="Duplissy, Jonathan" uniqKey="Duplissy J" first="Jonathan" last="Duplissy">Jonathan Duplissy</name><name sortKey="Ehrhart, Sebastian" sort="Ehrhart, Sebastian" uniqKey="Ehrhart S" first="Sebastian" last="Ehrhart">Sebastian Ehrhart</name><name sortKey="Kirkby, Jasper" sort="Kirkby, Jasper" uniqKey="Kirkby J" first="Jasper" last="Kirkby">Jasper Kirkby</name><name sortKey="Laaksonen, Ari" sort="Laaksonen, Ari" uniqKey="Laaksonen A" first="Ari" last="Laaksonen">Ari Laaksonen</name><name sortKey="Mathot, Serge" sort="Mathot, Serge" uniqKey="Mathot S" first="Serge" last="Mathot">Serge Mathot</name><name sortKey="Onnela, Antti" sort="Onnela, Antti" uniqKey="Onnela A" first="Antti" last="Onnela">Antti Onnela</name><name sortKey="Riccobono, Francesco" sort="Riccobono, Francesco" uniqKey="Riccobono F" first="Francesco" last="Riccobono">Francesco Riccobono</name><name sortKey="Trostl, Jasmin" sort="Trostl, Jasmin" uniqKey="Trostl J" first="Jasmin" last="Tröstl">Jasmin Tröstl</name><name sortKey="Virtanen, Annele" sort="Virtanen, Annele" uniqKey="Virtanen A" first="Annele" last="Virtanen">Annele Virtanen</name></country><country name="Finlande"><region name="Uusimaa"><name sortKey="Praplan, Arnaud P" sort="Praplan, Arnaud P" uniqKey="Praplan A" first="Arnaud P." last="Praplan">Arnaud P. Praplan</name></region><name sortKey="Adamov, Alexey" sort="Adamov, Alexey" uniqKey="Adamov A" first="Alexey" last="Adamov">Alexey Adamov</name><name sortKey="Duplissy, Jonathan" sort="Duplissy, Jonathan" uniqKey="Duplissy J" first="Jonathan" last="Duplissy">Jonathan Duplissy</name><name sortKey="Duplissy, Jonathan" sort="Duplissy, Jonathan" uniqKey="Duplissy J" first="Jonathan" last="Duplissy">Jonathan Duplissy</name><name sortKey="Franchin, Alessandro" sort="Franchin, Alessandro" uniqKey="Franchin A" first="Alessandro" last="Franchin">Alessandro Franchin</name><name sortKey="Hakala, Jani" sort="Hakala, Jani" uniqKey="Hakala J" first="Jani" last="Hakala">Jani Hakala</name><name sortKey="Jaeseok Kim" sort="Jaeseok Kim" uniqKey="Jaeseok Kim" last="Jaeseok Kim">JAESEOK KIM</name><name sortKey="Jokinen, Tuija" sort="Jokinen, Tuija" uniqKey="Jokinen T" first="Tuija" last="Jokinen">Tuija Jokinen</name><name sortKey="Junninen, Heikki" sort="Junninen, Heikki" uniqKey="Junninen H" first="Heikki" last="Junninen">Heikki Junninen</name><name sortKey="Kangasluoma, Juha" sort="Kangasluoma, Juha" uniqKey="Kangasluoma J" first="Juha" last="Kangasluoma">Juha Kangasluoma</name><name sortKey="Keskinen, Helmi" sort="Keskinen, Helmi" uniqKey="Keskinen H" first="Helmi" last="Keskinen">Helmi Keskinen</name><name sortKey="Kuimala, Markku" sort="Kuimala, Markku" uniqKey="Kuimala M" first="Markku" last="Kuimala">Markku Kuimala</name><name sortKey="Laaksonen, Ari" sort="Laaksonen, Ari" uniqKey="Laaksonen A" first="Ari" last="Laaksonen">Ari Laaksonen</name><name sortKey="Lawler, Michael J" sort="Lawler, Michael J" uniqKey="Lawler M" first="Michael J." last="Lawler">Michael J. Lawler</name><name sortKey="Lehtipalo, Katrianne" sort="Lehtipalo, Katrianne" uniqKey="Lehtipalo K" first="Katrianne" last="Lehtipalo">Katrianne Lehtipalo</name><name sortKey="Lehtipalo, Katrianne" sort="Lehtipalo, Katrianne" uniqKey="Lehtipalo K" first="Katrianne" last="Lehtipalo">Katrianne Lehtipalo</name><name sortKey="Pet J, Tuukka" sort="Pet J, Tuukka" uniqKey="Pet J T" first="Tuukka" last="Pet J">Tuukka Pet J</name><name sortKey="Rissanen, Matti P" sort="Rissanen, Matti P" uniqKey="Rissanen M" first="Matti P." last="Rissanen">Matti P. Rissanen</name><name sortKey="Sarnela, Nina" sort="Sarnela, Nina" uniqKey="Sarnela N" first="Nina" last="Sarnela">Nina Sarnela</name><name sortKey="Schobesberger, Siegfried" sort="Schobesberger, Siegfried" uniqKey="Schobesberger S" first="Siegfried" last="Schobesberger">Siegfried Schobesberger</name><name sortKey="Sipil, Mikko" sort="Sipil, Mikko" uniqKey="Sipil M" first="Mikko" last="Sipil">Mikko Sipil</name><name sortKey="Viisanen, Yrjo" sort="Viisanen, Yrjo" uniqKey="Viisanen Y" first="Yrjö" last="Viisanen">Yrjö Viisanen</name><name sortKey="Wimmer, Daniela" sort="Wimmer, Daniela" uniqKey="Wimmer D" first="Daniela" last="Wimmer">Daniela Wimmer</name><name sortKey="Worsnop, Douglas R" sort="Worsnop, Douglas R" uniqKey="Worsnop D" first="Douglas R." last="Worsnop">Douglas R. Worsnop</name></country><country name="Allemagne"><region name="Hesse (Land)"><name sortKey="Kurten, Andreas" sort="Kurten, Andreas" uniqKey="Kurten A" first="Andreas" last="Kürten">Andreas Kürten</name></region><name sortKey="Curtius, Joachim" sort="Curtius, Joachim" uniqKey="Curtius J" first="Joachim" last="Curtius">Joachim Curtius</name><name sortKey="Heinritzi, Martin" sort="Heinritzi, Martin" uniqKey="Heinritzi M" first="Martin" last="Heinritzi">Martin Heinritzi</name><name sortKey="Kirkby, Jasper" sort="Kirkby, Jasper" uniqKey="Kirkby J" first="Jasper" last="Kirkby">Jasper Kirkby</name><name sortKey="Leiminger, Markus" sort="Leiminger, Markus" uniqKey="Leiminger M" first="Markus" last="Leiminger">Markus Leiminger</name><name sortKey="Rondo, Linda" sort="Rondo, Linda" uniqKey="Rondo L" first="Linda" last="Rondo">Linda Rondo</name><name sortKey="Simon, Mario" sort="Simon, Mario" uniqKey="Simon M" first="Mario" last="Simon">Mario Simon</name><name sortKey="Williamson, Christina" sort="Williamson, Christina" uniqKey="Williamson C" first="Christina" last="Williamson">Christina Williamson</name><name sortKey="Wimmer, Daniela" sort="Wimmer, Daniela" uniqKey="Wimmer D" first="Daniela" last="Wimmer">Daniela Wimmer</name></country><country name="France"><noRegion><name sortKey="Ortega, Ismael K" sort="Ortega, Ismael K" uniqKey="Ortega I" first="Ismael K." last="Ortega">Ismael K. Ortega</name></noRegion></country><country name="Portugal"><noRegion><name sortKey="Amonm, Antonio" sort="Amonm, Antonio" uniqKey="Amonm A" first="Antonio" last="Amonm">Antonio Amonm</name></noRegion><name sortKey="Tome, Ant Nio" sort="Tome, Ant Nio" uniqKey="Tome A" first="Ant Nio" last="Tome">Ant Nio Tome</name></country><country name="Autriche"><noRegion><name sortKey="Breitenlechner, Martin" sort="Breitenlechner, Martin" uniqKey="Breitenlechner M" first="Martin" last="Breitenlechner">Martin Breitenlechner</name></noRegion><name sortKey="Breitenlechner, Martin" sort="Breitenlechner, Martin" uniqKey="Breitenlechner M" first="Martin" last="Breitenlechner">Martin Breitenlechner</name><name sortKey="Hansel, Armin" sort="Hansel, Armin" uniqKey="Hansel A" first="Armin" last="Hansel">Armin Hansel</name><name sortKey="Hansel, Armin" sort="Hansel, Armin" uniqKey="Hansel A" first="Armin" last="Hansel">Armin Hansel</name><name sortKey="Heinritzi, Martin" sort="Heinritzi, Martin" uniqKey="Heinritzi M" first="Martin" last="Heinritzi">Martin Heinritzi</name><name sortKey="Winkler, Paul M" sort="Winkler, Paul M" uniqKey="Winkler P" first="Paul M." last="Winkler">Paul M. Winkler</name></country><country name="États-Unis"><noRegion><name sortKey="Flagan, Richard C" sort="Flagan, Richard C" uniqKey="Flagan R" first="Richard C." last="Flagan">Richard C. Flagan</name></noRegion><name sortKey="Donahue, Neil M" sort="Donahue, Neil M" uniqKey="Donahue N" first="Neil M." last="Donahue">Neil M. Donahue</name><name sortKey="Lawler, Michael J" sort="Lawler, Michael J" uniqKey="Lawler M" first="Michael J." last="Lawler">Michael J. Lawler</name><name sortKey="Penglin Ye" sort="Penglin Ye" uniqKey="Penglin Ye" last="Penglin Ye">PENGLIN YE</name><name sortKey="Worsnop, Douglas R" sort="Worsnop, Douglas R" uniqKey="Worsnop D" first="Douglas R." last="Worsnop">Douglas R. Worsnop</name></country><country name="Russie"><region name="District fédéral central"><name sortKey="Makhmutov, Vladimir" sort="Makhmutov, Vladimir" uniqKey="Makhmutov V" first="Vladimir" last="Makhmutov">Vladimir Makhmutov</name></region></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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